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    Items for Author "Hsieh, C. H."  

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    Showing 66 items.

    Collection Date Title Authors Bitstream
    [化學學系暨研究所] 會議論文 2018-03-18 Triplet, high-​spin, linear {Fe(NO)​}​8: Redox feature of a stable diiron trinitrosyl complex Ghosh, Pokhraj; Ding, Shengda; Quiroz, Manuel; Hsieh, Chung-Hung; Hall, Michael B.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2018-03-18 Metallodithiolate ligands as pendant base in [FeIFeI]​, [FeI[Fe(NO)​]​II] and [(μ-​H)​FeIIFeII] systems Kariyawasam Pathirana, Kavindu Dilshan; Ghosh, Pokhraj; Hsieh, Chung-Hung; Bhuvanesh, Nattamai; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2017-04-02 Unleashing a pendant base by reduction-​induced hemilability in [NiN2S2.Fe(NO)​2]​+​/0 complexes Ghosh, Pokhraj; Ding, Shengda; Hsieh, Chung-Hung; Chupik, Rachel B.; Bhuvanesh, Nattamai S.; Hall, Michael B.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2016-11-09 Dinitrosyl iron units as redox markers to generate synthetic analogues of [NiFe]​-​hydrogenase enzyme active site Ghosh, Pokhraj; Chupik, Rachel B.; Hsieh, Chung-Hung; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2016-08-21 Advances in the preparation of redox active NiFe complexes based on NiN2S2-​Fe(NO)​2 as synthetic analogues of [NiFe]​-​hydrogenase enzyme active site Ghosh, Pokhraj; Ding, Shengda; Hsieh, Chung-Hung; Chupik, Rachel B.; Bhuvanesh, Nattamai S.; Hall, Michael B.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2016-03-13 Comparison of S-​H bond vs. S-​Au bond beyond the isolobal relationship between proton and gold-​phosphine anion Ding, Shengda; Crouthers, Danielle; Denny, Jason; Bethel, Ryan D.; Hsieh, Chung-Hung; Hall, Michael B.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2014-08 Carbon monoxide induced elimination of disulfide from dinitrosyl iron complexes: Hammett correlations of para-substituted [(NHC)Fe(NO)2S(p-PhX)] compounds Pulukkody, Randara; Kyran, Samuel; Drummond, Michael; Hsieh, Chung-Hung; Bethel, Ryan; Darensbourg, Donald J.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2014-03 Further mechanistic studies of carbon monoxide induced reductive elimination of disulfide in N-heterocyclic carbene (NHC)/thiolate dinitrosyl iron complexes (DNICs) Drummond, Michael J.; Pulukkody, Randara; Kyran, Samuel J.; Hsieh, Chung Hung; Darensbourg, Donald J.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2013-11 Iron-nitrosyl paradigm for base metal proton reduction electrocatalysis Darensbourg, Marcetta Y.; Hsieh, Chung-hung; Erdem, Ozlen; Ding, Shengda; Crouthers, Danielle; Lubitz, Wolfgang; Popescu, Codrina; Reibenspies, Joseph; Hall, Michael B.
    [化學學系暨研究所] 會議論文 2013-11 A NEW MEMBER OF TETRANUCLEAR DINITROSYL IRON COMPLEXES 謝忠宏
    [化學學系暨研究所] 會議論文 2013-04 Ambidentate thiocyanate ligand in dinitrosyl iron complexes Hsieh, Chung-Hung; Brothers, Scott M.; Hall, Michael B.; Popescu, Codrina V.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2013-04 Cis-NiN2S2 metallodithiolates as mono- and bidentate S-donors to gold (I) Pinder, Tiffany A.; Montalvo, Steven K.; Lunsford, Allen M.; Hsieh, Chung-Hung; Reibenspies, Joseph H.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2013-04 Dinitrosyl iron adducts of (N2S2)M(NO) complexes (M=Ni, Fe, Co) as metallodithiolate ligands Chupik, Rachel B.; Hsieh, Chung-Hung; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2013-04 Electronic effects of metallodithiolate ligands on [FeFe]-H2ase active site model compounds Ghosh, Pokhraj; Hsieh, Chung-Hung; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2013-04 Ligand-assisted proton delivery in diiron complexes as electrocatalysts for H2 production: Ligand and complex synthesis Zaibaq, Nicholas; Ghosh, Pokhraj; Hsieh, Chung-Hung; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2013-04 N2S2-nickel and iron nitrosyls as metallo ligands in synthetic analogs of the [FeFe]-H2ase enzyme active site Darensbourg, Marcetta Y.; Hsieh, Chung-Hung; Ghosh, Pokhraj
    [化學學系暨研究所] 會議論文 2013-04 Structural and spectroscopic features of mixed valent FeIIFeI complexes and factors related to the rotated configuration of diiron hydrogenase Hsieh, Chung-Hung; Erdem, Ozlen; Harman, Scott; Singleton, Michael; Reijerse, Edward; Lubitz, Wolfgang; Popescu, Codrina; Reibenspies, Jospeh; Brothers, Scott; Hall, Michael; et a
    [化學學系暨研究所] 會議論文 2012-08 Base-promoted tautomerization of imidazoles to N-heterocyclic carbenes (NHCs): Via a dinitrosyl iron scaffold Hsieh, Chung-Hung; Pulukkody, Randara; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2012-08 Critical precursors to biomimetics of the diiron hydrogenase enzyme active site: Carbon monoxide mobilized 2Fe2S carbonyl clusters Darensbourg, Marcetta Y.; Crouthers, Danielle; Bethel, Ryan; Hsieh, Chung-Hung; Brothers, Scott M.; Hall, Michael B.
    [化學學系暨研究所] 會議論文 2012-08 Moessbauer studies of mixed-valence Fe(II)Fe(I) and Fe(I)Fe(I) model complexes illustrating states of the H-cluster in [Fe-Fe]-hydrogenases Popescu, Codrina V.; Darensbourg, Marcetta Y.; Hsieh, Chung-Hung; Stoian, Sebastian A.; Casuras, Andrea
    [化學學系暨研究所] 會議論文 2012-08 Moessbauer studies of model complexes for the H-cluster in [Fe-Fe]-hydrogenases: Electronic structure of mixed-valence complexes containing low-spin Fe(I) Popescu, Codrina V.; Stoian, Sebastian A.; Hsieh, Chung-Hung; Darensbourg, Marcetta Y.; Casuras, Andrea
    [化學學系暨研究所] 會議論文 2012-08 Paramagnetic transition metal ions in N2S2 coordination Pinder, Tiffany A.; Hsieh, Chung-Hung; Lunsford, Allen M.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2012-08 Rich man's proton: Triphenylphosphinegold as probe of hydride positions in organo- and bioorgano-metallic complexes Darensbourg, Marcetta Y.; Hsieh, Chung-Hung; Brothers, Scott; Hall, Michael B.
    [化學學系暨研究所] 會議論文 2012-03 When iron meets nitric oxide: Good chemistry, intriguing biology Darensbourg, Marcetta Y.; Hsieh, Chung-Hung; Hess, Jennifer L.; Brothers, Scott; Hall, Michael B.
    [化學學系暨研究所] 會議論文 2011-11 The vanadyl ion in N2S2 coordination Pinder, Tiffany A.; Jenkins, Roxanne M.; Hsieh, Chung-Hung; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 會議論文 2011-03 Synthesis, characterization, and reactivity of dinitrosyl iron complexes stabilized by N-heterocyclic carbenes Hess, Jennifer L.; Hsieh, Chung-Hung; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2019 Frontier chemistry and materials for 21st century, No. 3: preface San-Lang Wang; Po-Shen Pan; Chung-Hung Hsieh
    [化學學系暨研究所] 期刊論文 2018-09-14 Structural and Electronic Responses to the Three Redox Levels of Fe(NO)​N2S2-​Fe(NO)​(2) Ghosh, Pokhraj; Ding, Shengda; Quiroz, Manuel; Bhuvanesh, Nattamai; Hsieh, Chung-Hung; Palacios, Philip M.; Pierce, Brad S.; Darensbourg, Marcetta Y.; Hall, Michael B.
    [化學學系暨研究所] 期刊論文 2017-10-12 A matrix of heterobimetallic complexes for interrogation of hydrogen evolution reaction electrocatalysts Ghosh,Pokhraj; Ding,Shengda; Chupik,Rachel B.; Quiroz,Manuel; Hsieh,Chung-Hung; Bhuvanesh,Nattami; Hall,Michael B.; Darensbourg,Marcetta Y
    [化學學系暨研究所] 期刊論文 2017-06-01 Synthesis of five-coordinate manganese(I) carbonyl complex [(CO)3Mn (-S,-Se-C6H3-4-Me)]-: influences of non-innocent ligand to the structure, reactivity and electrochemical property Chen, Chien-Hong; Hung, Shih-Hsuan; Du, Wan-Ting; Hsieh, Chung-Hung
    [化學學系暨研究所] 期刊論文 2016-03-17 Synthesis and stability study of isocyano aryl boronate esters and their synthetic applications Hao-Ping Fang; Chia-Chieh Fu; Chin-Kuen Tai; Ken-Hao Chang; Ru-Han Yang; Meng-Ju Wu; Hsien-Chi Chen; Chia-Jung Li; Shi-Qing Huang; Wan-Hsiang Lien; Chih-Hsin Chen; Chung-Hung Hsieh; Bo-Cheng Wang; Siu-Fung Cheung; Po-Shen Pan
    [化學學系暨研究所] 期刊論文 2015-09-14 A Reduced 2Fe2S Cluster Probe of Sulfur-​Hydrogen versus Sulfur-​Gold Interactions Crouthers, Danielle J.; Ding, Shengda; Denny, Jason A.; Bethel, Ryan D.; Hsieh, Chung-Hung; Hall, Michael B.; Darensbourg, Marcetta Y
    [化學學系暨研究所] 期刊論文 2015-03-13 Regioselectivity in Ligand Substitution Reactions on Diiron Complexes Governed by Nucleophilic and Electrophilic Ligand Properties Bethel, Ryan D.; Crouthers, Danielle J.; Hsieh, Chung-Hung; Denny, Jason A.; Hall, Michael B.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2014-10 Hammett correlations as test of mechanism of CO-induced disulfide elimination from dinitrosyl iron complexes Randara Pulukkody; Samuel J. Kyran; Michael J. Drummond; Hsieh, Chung-Hung; Donald J. Darensbourg; Marcetta Y. Darensbourg; Marcetta Y. Darensbourg
    [化學學系暨研究所] 期刊論文 2014-07-01 A new member of tetranuclear dinitrosyl iron complexes (DNICs) with 2-mercaptothiazoline ligand: synthesis, structure and properties Hsieh, Chung-Hung; Chen, Chien-Hong; Wang, Jheng-Hong; Huang, Jing-Yi; Chen, Chien-Hong; Hsieh, Chung-Hung
    [化學學系暨研究所] 期刊論文 2014-05-02 Redox active iron nitrosyl units in proton reduction electrocatalysis Hsieh, Chung-Hung; Shengda Ding; Özlen F. Erdem; Danielle J. Crouthers; Tianbiao Liu; Charles C. L. McCrory; Wolfgang Lubitz; Codrina V. Popescu; Joseph H. Reibenspies; Michael B. Hall; Marcetta Y. Darensbourg; Marcetta Y. Darensbourg
    [化學學系暨研究所] 期刊論文 2014-01-01 Versatile N2S2 nickel-dithiolates as mono- and bridging bidentate, S-donor ligands to gold(I) Pinder Tiffany A.; Montalvo Steven K.; Lunsford Allen M.; Hsieh, Chung-Hung; Reibenspies Joseph H.; Darensbourg Marcetta Y.; Darensbourg Marcetta Y.
    [化學學系暨研究所] 期刊論文 2014-01-01 Metallodithiolates as Ligands to Dinitrosyl Iron Complexes: Toward the Understanding of Structures, Equilibria, and Spin Coupling Pinder Tiffany A.; Montalvo Steven K.; Hsieh, Chung-Hung; Lunsford Allen M.; Bethel Ryan D.; Pierce Brad S; Darensbourg Marcetta Y.; Darensbourg Marcetta Y.
    [化學學系暨研究所] 期刊論文 2013-08-16 A dinitrosyl iron complex as a platform for metal-bound imidazole to N-heterocyclic carbene conversion Hsieh, Chung-Hung; Pulukkody, Randara; Darensbourg, Marcetta Y.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2013-08 Hyperfine interactions and electron distribution in Fe(II)Fe(I) and Fe(I)Fe(I) models for the active site of the [FeFe] hydrogenases: Mössbauer spectroscopy studies of low-spin Fe(I) Stoian Sebastian A.; Hsieh, Chung-Hung; Singleton Michael L.; Casuras Andrea F.; Darensbourg Marcetta Y.; McNeely Kelsey; Sweely Kurt; Popescu Codrina V.; Popescu Codrina V.
    [化學學系暨研究所] 期刊論文 2013-07 Dinitrosyl iron adducts of (N2S2)M(NO) complexes (M = Fe, Co) as metallodithiolate ligands Hsieh, Chung-Hung; Chupik, Rachel B.; Pinder, Tiffany A.; Darensbourg, Marcetta Y.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2013-06-07 Bridging-hydride influence on the electronic structure of an [FeFe] hydrogenase active-site model complex revealed by XAES-DFT Leidel, Nils; Hsieh, Chung-Hung; Chernev, Petko; Sigfridsson, Kajsa G. V.; Darensbourg, Marcetta Y.; Haumann, Michael
    [化學學系暨研究所] 期刊論文 2013-06-01 Carbon Monoxide Induced Reductive Elimination of Disulfide in an N-Heterocyclic Carbene (NHC)/ Thiolate Dinitrosyl Iron Complex (DNIC) Pulukkody, Randara; Kyran, Samuel J.; Bethel, Ryan D.; Hsieh, Chung-Hung; Hall, Michael B.; Darensbourg, Donald J.; Darensbourg, Marcetta Y.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2013-02-01 Ambidentate Thiocyanate and Cyanate Ligands in Dinitrosyl Iron Complexes Hsieh, Chung-Hung; Brothers, Scott M.; Reibenspies, Joseph H.; Hall, Michael B.; Popescu, Codrina V.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2012-08-01 Structural and Spectroscopic Features of Mixed Valent Fe(II)Fe(I) Complexes and Factors Related to the Rotated Configuration of Diiron Hydrogenase Hsieh, Chung-Hung; Erdem, Ozlen F.; Harman, Scott D.; Singleton, Michael L.; Reijerse Edward; Lubitz Wolfgang; Popescu, Codrina V.; Reibenspies Joseph H.; Brothers Scott M.; Hall Michael B.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2011-12 Self-Assembly of Dinitrosyl Iron Units into Imidazolate-Edge-Bridged Molecular Squares: Characterization Including Mössbauer Spectroscopy Hess, Jennifer L.; Hsieh, Chung-Hung; Brothers, Scott M.; Hall, Michael B.; Darensbourg, Marcetta Y.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2011-09 N-Heterocyclic Carbene Ligands as Mimics of Imidazoles/Histidine for the Stabilization of Di- and Trinitrosyl Iron Complexes Hess, Jennifer L.; Hsieh, Chung-Hung; Reibenspies, Joseph H.; Darensbourg, Marcetta Y.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2011-05 cis-Dithiolatonickel as metalloligand to dinitrosyl iron units: the di-metallic structure of Ni(l-SR)[Fe(NO)2] and an unexpected, abbreviated metalloadamantyl cluster, Ni2(l-SR)4[Fe(NO)2]3 Hsieh, Chung-Hung; Chupik, Rachel B.; Brothers, Scott M.; Hall, Michael B.; Darensbourg, Marcetta Y.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2010-10 A {Fe(NO)3}10 Trinitrosyliron Complex Stabilized by an N-Heterocyclic Carbene and the Cationic and Neutral {Fe(NO)2}9/10 Products of Its NO Release Hsieh, Chung-Hung; Darensbourg Marcetta Y.; Darensbourg Marcetta Y.
    [化學學系暨研究所] 期刊論文 2008-08 Nitric Oxide Physiological Responses and Delivery Mechanisms Probed by Water-Soluble Roussin’s Red Ester and {Fe(NO)2}10 DNIC Chen, Yi-Ju; Ku, Wei-Chi; Feng, Li-Ting; Tsai, Ming-Li; Hsieh, Chung-Hung; Hsu, Wen-Hwei; Liaw, Wen-Feng; Hung, Chen-Hsiung; Chen, Yu-Ju
    [化學學系暨研究所] 期刊論文 2007-08 A reduced 2Fe2S cluster probe of sulfur-hydrogen versus sulfur-gold interactions Crouthers, Danielle J.; Ding, Shengda; Denny, Jason A.; Bethel, Ryan D.; Hsieh, Chung-Hung; Hall, Michael B.; Darensbourg, Marcetta Y.
    [化學學系暨研究所] 期刊論文 2007-06 Dinitrosyl Iron Complexes (DNICs) Containing S/N/O Ligation: Transformation of Roussin's Red Ester into the Neutral {Fe(NO)2}10 DNICs Tsai, Ming-Li; Hsieh, Chung-Hung; Liaw, Wen-Feng; Liaw, Wen-Feng
    [化學學系暨研究所] 期刊論文 2007-02 New Members of a Class of Iron−Thiolate−Nitrosyl Compounds: Trinuclear Iron−Thiolate−Nitrosyl Complexes Containing Fe3S6 Core Hsu, I-Jui; Hsieh, Chung-Hung; Ke, Shyue-Chu; Chiang, Kuo-An; Lee, Jenn-Min; Chen, Jin-Ming; Jang, Ling-Yun; Lee, Gene-Hsiang; Wang, Yu; Liaw, Wen-Feng
    [化學學系暨研究所] 期刊論文 2004-08 Photochemistry of the Dinitrosyl Iron Complex [S5Fe(NO)2]- Leading to Reversible Formation of [S5Fe(μ-S)2FeS5]2-: Spectroscopic Characterization of Species Relevant to the Nitric Oxide Modification and Repair of [2Fe−2S] Ferredoxins Tsai, Ming-Li; Chen, Chiao-Chun; Hsu, I-Jui; Ke, Shyue-Chu; Hsieh, Chung-Hung; Chiang, Kuo-An; Lee, Gene-Hsiang; Wang, Yu; Chen, Jin-Ming; Lee, Jyh-Fu; Liaw, Wen-Feng
    [化學學系暨研究所] 期刊論文 2003-09 Oxygen Binding to Sulfur in Nitrosylated Iron−Thiolate Complexes:  Relevance to the Fe-Containing Nitrile Hydratases Lee, Chien-Ming; Hsieh, Chung-Hung; Dutta Amitava; Lee, Gene-Hsiang; Liaw, Wen-Feng
    [化學學系暨研究所] 期刊論文 2003-06 Nickel Complexes of o-Amidochalcogenophenolate(2−)/o-Iminochalcogenobenzosemiquinonate(1−) π-Radical: Synthesis, Structures, Electron Spin Resonance, and X-ray Absorption Spectroscopic Evidence Hsieh, Chung-Hung; Hsu, I-Jui; Lee, Chien-Ming; Ke, Shyue-Chu; Wang, Tze-Yuan; Lee, Gene-Hsiang; Wang, Yu; Chen, Jin-Ming; Lee, Jyh-Fu; Liaw, Wen-Feng
    [化學學系暨研究所] 期刊論文 2003-03 無機生物配位化學 Chen, Chien-Hong; Lee, Chien-Ming; Hsieh, Chung-Hung; Liaw, Wen-Feng
    [化學學系暨研究所] 期刊論文 2003-02 Effect of Ca2+ and La3+ in Y1-xCaxBa2-xLaxCu3Oy study : an X-ray absorption spectroscopy Hsieh, C. H.; Chang, C. N.; Lee, S. B.; 高惠春; Kao, H. C. I.; Chin, C. H.
    [化學學系暨研究所] 期刊論文 2003-02 Evidence of the effect of the apical oxygen on the superconductivity of Y1−xCaxBa2Cu3Oy. An O-1s X-ray absorption spectroscopy study Hsieh, C. H.; Chang, C.N.; Lee, S. B.; Kao, H.-C. I.; Chin, C. H.; Chang, C. N.
    [化學學系暨研究所] 期刊論文 2002-04 S-S Bond-activation of diorganyl disulfide by anionic [Mn(CO)5]-: crystal structures of [MnII(-SC5H4NO-)3]- and [(CO)3Mn(μ-SR)3Co(μ-SR)3Mn(CO)3]- (R = C6H4NHCOPh) Liaw, Wen-Feng; Hsieh, Chung-Hung; Peng, Shie-Ming; Lee, Gene-Hsiang; Liaw, Wen-Feng
    [化學學系暨研究所] 期刊論文 2000-10-31 X-ray absorption study of YBa2−xLaxCu3Oy Hsieh, C.H.; Chang, C.N.; Lee, S.B.; Kao, H.-C.I.; Chin, C.H.; Chang, C.N.
    [化學學系暨研究所] 期刊論文 1999-08 O-1s x-ray near-edge absorption spectroscopy studies of La1.5-xCaxBa1.5Cu3Oy and La1.5CaxBa1.5-xCu3Oy Song, Y. F.; Chang, C. N.; Kao, H.-C. I.; Hsieh, C. H.; Liu, H. F.; Lin, H. D.; Huang, W. W.
    [化學學系暨研究所] 期刊論文 1999-02 The energy shift and the hole localization in Y1-xPrxBa2Cu3O7-δ from O ls x-ray near-edge-absorption spectroscopy study Chang, C. N.; Song, Y. F.; Hsieh, C. H.; Liu, H. F.; 高惠春; Kao, H. C. I.; Yang, H. C.
    [化學學系暨研究所] 期刊論文 1999 A five-coordinate, sixteen-electron manganese(I) complex [Mn(CO)3(S,S–C6H4)]– stabilized by S,S π-donation from chelating [S,S–C6H4]2– Lee, Chien-Ming; Lin, Ging-Yi; Hsieh, Chung-Hung; Hu, Ching-Han; Lee, Gene-Hsiang; Peng, Shie-Ming; Liaw, Wen-Feng
    [物理學系暨研究所] 期刊論文 1998-03 A low-cost and flexible double-crystal monochromator for an x-ray beamline Hwang, C. S.; Lin, F. Y.; Lee, Chih-Hao; Yu, Kuan-li; Hsieh, C. H.; 鄭伯昆; Tseng, P. K.; Lin, J. T.; 彭維鋒; Pong, W. F.
    [物理學系暨研究所] 期刊論文 1998-03 A low cost and flexible double crystal monochronator for X-Ray beamline Hwang, C.S.; Lin, F.Y.; Lee, C.H.; Yu, K.L.; Hsieh, C.H.; Tseng, P.K.; Lin, J.T.; 彭維鋒; Pong, Way-faung

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