Abstract: | A new series of spin-crossover octahedral Fe(II) complexes with the composition Fe (II) (N-R-2-pyridinaldimine)2(NCS)2, where, R=phenyl, naphthalenyl,cyclohexyl, anthracenyl, pyrenyl, 1,2,3,4-tetrahydro-1-naphthalenyl, 5,6,7,8,-tetrahedro-1-naphthalenyl, benzyl, 1-phenylethyl, 1-phenylpropyl, have been synthesized and their spin states of iron atom have been studied by means of Mőssbauer spectrscopy. |