Nickel-Catalyzed Intramolecular Dual Annulation Reaction of Aryl Nitrile-Containing 1,2,3-Benzotriazin-4(3H)‑ones: A Pathway To Synthesize Luotonin A and Related Polycyclic Pyrroloquinazolinones

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题名:	Nickel-Catalyzed Intramolecular Dual Annulation Reaction of Aryl Nitrile-Containing 1,2,3-Benzotriazin-4(3H)‑ones: A Pathway To Synthesize Luotonin A and Related Polycyclic Pyrroloquinazolinones
作者:	Thorat, Vijaykumar H.;Hsieh, Jen-Chieh
日期:	2023-10-31
上传时间:	2024-07-10 12:05:40 (UTC+8)
出版者:	ACS Publications
摘要:	Herein, we report a nickel-catalyzed intramolecular denitrogenative dual annulation reaction of aryl nitrile-containing 1,2,3-benzotriazine-4(3H)-ones to synthesize polycyclic pyrroloquinazolinones with a tolerance of a wide diversity of substituents. This catalytic reaction is the first denitrogenative transannulation of 1,2,3-benzotriazine-4(3H)-one with nitrile, which can be applied as the critical step to synthesize luotonin A with a high step economy.
關聯:	Organic Letters, 25(44), p.7990-7994
DOI:	10.1021/acs.orglett.3c03142
显示于类别:	[化學學系暨研究所] 期刊論文

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