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| 題名: | Nickel-Catalyzed Intramolecular Dual Annulation Reaction of Aryl Nitrile-Containing 1,2,3-Benzotriazin-4(3H)‑ones: A Pathway To Synthesize Luotonin A and Related Polycyclic Pyrroloquinazolinones |
| 作者: | Thorat, Vijaykumar H.;Hsieh, Jen-Chieh |
| 日期: | 2023-10-31 |
| 上傳時間: | 2024-07-10 12:05:40 (UTC+8) |
| 出版者: | ACS Publications |
| 摘要: | Herein, we report a nickel-catalyzed intramolecular denitrogenative dual annulation reaction of aryl nitrile-containing 1,2,3-benzotriazine-4(3H)-ones to synthesize polycyclic pyrroloquinazolinones with a tolerance of a wide diversity of substituents. This catalytic reaction is the first denitrogenative transannulation of 1,2,3-benzotriazine-4(3H)-one with nitrile, which can be applied as the critical step to synthesize luotonin A with a high step economy. |
| 關聯: | Organic Letters, 25(44), p.7990-7994 |
| DOI: | 10.1021/acs.orglett.3c03142 |
| 顯示於類別: | [化學學系暨研究所] 期刊論文
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