淡江大學機構典藏:Item 987654321/124090
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    题名: Nematic electron and phonon dynamics in SnS crystals
    作者: Hsueh, Hung-chung
    关键词: Phonons;Nonequilibrium thermodynamics;2D materials;Ultrafast phenomena;Photoexcitations;Pump probe spectroscopy
    日期: 2022-10-24
    上传时间: 2023-05-15 12:05:34 (UTC+8)
    出版者: AIP (美國物理協會)
    摘要: Tin sulfide (SnS) is one of the promising materials for the applications of optoelectronics and photovoltaics. This study determines the
    nematic dynamics of photoexcited electrons and phonons in SnS single crystals using polarization-dependent pump–probe spectroscopy at
    various temperatures. As well as the fast (0.21–1.38 ps) and slow (>5 ps) relaxation processes, a 36–41 GHz coherent acoustic phonon with a
    sound velocity of 4883 m/s that is generated by the thermoelastic effect is also observed in the transient reflectivity change (DR/R) spectra.
    Electrons and coherent acoustic phonons show significant in-plane anisotropy from 330 to 430 K due to strong electron–phonon coupling.
    However, this in-plane anisotropy weakens dramatically in the low-temperature (<330 K) and high-temperature (>430 K) phases. These
    results add to the knowledge about the anisotropy of electrons and coherent acoustic phonons that give SnS applications in photovoltaic or
    optoelectronic devices.
    關聯: Applied Physics Letters 121(17)
    DOI: 10.1063/5.0099486
    显示于类别:[Graduate Institute & Department of Physics] Journal Article

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