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    题名: Infrared Nonlinear Optical Polymorphs α- and β-SrCu2SnS4 Exhibiting Large Second Harmonic Generation Responses with Requisite Phase-Matching Behavior
    作者: Yang, Ya;Wu, Kui;Zhang, Bingbing;Wu, Xiaowen;Lee, Ming-Hsien
    日期: 2020-01-21
    上传时间: 2020-06-01 12:13:52 (UTC+8)
    摘要: α- and β-SrCu2SnS4 polymorphs, exhibiting special structural changes and excellent physicochemical performances, were successfully synthesized and characterized as promising IR NLO candidates. Note that they satisfy the essential phase-matching condition and have strong SHG responses about 0.7 and 1.0 times those of benchmark AgGaS2 under 2.09 μm incident light, respectively, which agree well with the theoretical SHG coefficients and suitable birefringences based on first-principles calculation. Moreover, it is also verified that their SHG effects originate from the synergetic contribution between CuS4 and SnS4 ligands after the SHG density calculations.
    關聯: CHEMISTRY OF MATERIALS 32(3), p.1281-1287
    DOI: 10.1021/acs.chemmater.9b04842
    显示于类别:[物理學系暨研究所] 期刊論文

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