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    題名: Multi-objective Optimization of Mixed Membrane Reactors for Autothermal Reforming of Methane
    作者: Hsuan Chang;Yih-Hung Chen;Yun-Tsz Chen;Chii-Dong Ho
    關鍵詞: Methane Reforming;Membrane Reactor;Mixed Membrane Reactor;Multi-objective Optimization
    日期: 2018-09
    上傳時間: 2018-11-01 12:11:18 (UTC+8)
    出版者: 淡江大學
    摘要: Autothermal reforming (ATR) of methane, which supplies the heat for endothermic steam reforming by internal combustion of methane, is an important process for synthetic gas production. The axial-distributed feeding of oxygen via a packed bed inert membrane reactor (MR) can reduce the peak temperature and improve the reactor performance. A modified MR, called mixed membrane reactor (MMR), combines permeable membrane tube wall and non-permeable tube wall provides extra degrees of freedom for reactor design and operation. For MR and MMR, this study presents the ternary-objective optimization analysis for maximizing hydrogen production rate, non-combustion selectivity and conversion of methane, using a 1D pseudo-homogeneous reactor model and the NSGA-II algorithm. Compared to MR, MMR can be operated under significantly higher oxygen permeation flux without violating the maximum temperature constraint. The non-combustion selectivity and conversion of methane of MR and MMR are close, however, the hydrogen production rate of MMR can be as high as 200% of MR.
    關聯: 淡江理工學刊 21(3), p.485-495
    DOI: 10.6180/jase.201809_21(3).0020
    顯示於類別:[化學工程與材料工程學系暨研究所] 期刊論文


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