Uranium oxide nanocrystals by microwave-assisted thermal decomposition: electronic and structural properties

淡江大學機構典藏 > 理學院 > 物理學系暨研究所 > 期刊論文 > Item 987654321/113665

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题名:	Uranium oxide nanocrystals by microwave-assisted thermal decomposition: electronic and structural properties
作者:	Jennifer Leduc;Joseph I. Pacold;David K. Shuh;Chung‐Li Dong;Sanjay Mathur
关键词:	In‐situ X‐ray absorption spectroscopy;Scanning transmission X‐ray microscopy (STXM);Photocatalysis;Uranium;UO 2 nanoparticles;Microwave chemistry
日期:	2017-11-14
上传时间:	2018-06-08 12:10:12 (UTC+8)
出版者:	Wiley
摘要:	Uranium oxides have attracted much attention not only in the context of nuclear energy generation but also for their application as pristine catalysts or as supports for other (transition metal) oxides and (precious) metals. Their propensity to adopt high coordination numbers and manifest multiple oxidation states (from +II to +VI) makes them attractive candidates for catalyzed transformation reactions. Herein, we report a new synthesis route to phase‐pure, crystalline UO2 nanoparticles via microwave‐assisted decomposition of a molecular uranium(IV) precursor. The electronic structure and optical absorption properties of these nanocrystals were investigated using spectroscopic methods to evaluate their suitability for photo(electro)catalytic applications.
關聯:	Zeitschrift für anorganische and allgemeine Chemie 644(1), p.12-18
DOI:	10.1002/zaac.201700294
显示于类别:	[物理學系暨研究所] 期刊論文

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